Metallica (Master of Puppets, 'cause it's from DOOM!!! ).
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How much of their stuff have you listened to? Master of Puppets is definitely a great one. Find the Live version! That's one of their best live songs, in my opinion.
I could name a ton of songs by Metallica that are really good. Of all of the bands I've ever listened to, they've got the most good songs. I'll just give you a run down of my favorite songs of theirs:
Kill 'Em All
(Unlike most Metallica fans, I don't really care for any of the stuff from their first album, Kill 'Em All. At least, none of the songs on that album stand out as "favorites" of mine. I have the album in my playlist, but don't care for it a ton.)
Ride the Lightning
For Whom the Bell Tolls
Fade to Black
Trapped Under Ice
The Call of Ktulu
Master of Puppets
Battery
Master of Puppets
The Thing That Should Not Be
Welcome Home (Sanitarium)
Disposable Heroes
...And Justice for All
Blackened
...And Justice for All
Eye of the Beholder
One
Harvester of Sorrow
To Live Is to Die
Metallica
The entire Album. It's just that good.
Enter Sandman (I don't care much for it myself, honestly, because it's overdone, but it's a great song either way, I'm just sick of it myself)
Sad But True
Holier Than Thou
The Unforgiven
Wherever I May Roam
Don't Tread on Me
Through the Never
Nothing Else Matters
Of Wolf and Man
The God That Failed
My Friend of Misery
The Struggle Within
Load
Ain't My Bitch
Until It Sleeps
King Nothing
Bleeding Me
Mama Said
The Outlaw Torn
ReLoad
Fuel
The Memory Remains
Devil's Dance
The Unforgiven II
Better Than You
Carpe Diem Baby
St. Anger
(Unlike most Metallica fans, I actually like a lot of this album. Most people seem to think it's horrible. If you don't directly compare it to their older stuff, it's still better than 95% of what else is out there.)
Frantic
St. Anger
Some Kind of Monster
Invisible Kid
My World
Shoot Me Again
Sweet Amber
The Unnamed Feeling
Purify
All Within My Hands
You might wanna check out System of a Down, as well. They're a bit spastic sometimes, but if you can tolerate that, they're pretty damn unique, and they have a lot of good messages as well.